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I'm not sure this is exactly what you're asking for, but I found this old MAPDL input file that uses two spring elements (COMBIN14 and COMBIN39) to posit nonlinear negative stiffness between two nodes (to mimic net magnetic force versus separation):
Note that as node 2 at the bottom of the two element model is moved upward, the reaction force becomes increasingly negative (the springs are pulling upward on node 2 with increasing force as node 2 gets closer to node 3).
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In Mechanical, you would have to include commands like these in a command object, maybe written in such a way that the springs are attached to remote point nodes scoped to surfaces.
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--Bill