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Hi Vu Vuong,
Please note that you can enter these measured values as relative permittivity and dielectric loss tangent properties for a custom material in HFSS. Please go through the "Materials Technical Notes" section of the HFSS Help document for detailed information on how to correlate the measured values in terms of relative permittivity and dielectric loss tangent properties.
As you have frequency dependency then you need to add these properties as data sets. Detailed information on how to enter frequency dependent data sets can be found in "Assigning Frequency Dependent Material: Enter Frequency Dependent Data Points" section of the HFSS Help document.
Best regards,
Praneeth.